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Substrate-Induced Carbon Monoxide Reactivity Suggests Multiple Enzyme Conformations at the Catalytic Copper M-Center of Peptidylglycine Monooxygenase

The present study uses CO as a surrogate for oxygen to probe how substrate binding triggers oxygen activation in peptidylglycine monooygenase (PHM). Infrared stretching frequencies (ν(C≡O)) of the carbonyl (CO) adducts of copper proteins are sensitive markers of Cu(I) coordination, and are useful in...

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Publicat a:Biochemistry
Autors principals: Kline, Chelsey D, Blackburn, Ninian J
Format: Artigo
Idioma:Inglês
Publicat: 2016
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC5161237/
https://ncbi.nlm.nih.gov/pubmed/27933800
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.biochem.6b00845
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