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Enantioselective Formation of All-Carbon Quaternary Centers via C–H Functionalization of Methanol: Iridium-Catalyzed Diene Hydrohydroxymethylation
The first catalytic enantioselective C-C couplings of methanol (> 30× 10(6) tons/year) are reported. Formal insertion of 2-substituted dienes into the methanol C–H bond occurs in a regioselective manner to form all-carbonyl quaternary centers with excellent levels of enantioselectivity using an i...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5094804/ https://ncbi.nlm.nih.gov/pubmed/27762549 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b09333 |
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