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An Fe-N(2) Complex That Generates Hydrazine and Ammonia via Fe═NNH(2): Demonstrating a Hybrid Distal-to-Alternating Pathway for N(2) Reduction
Biological N(2) fixation to NH(3) may proceed at one or more Fe sites in the active-site cofactors of nitrogenases. Modeling individual e(−)/H(+) transfer steps of iron-ligated N(2) in well-defined synthetic systems is hence of much interest but remains a significant challenge. While molecular Fe sp...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5065353/ https://ncbi.nlm.nih.gov/pubmed/26937584 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b01230 |
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