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N–H Bond Dissociation Enthalpies and Facile H Atom Transfers for Early Intermediates of Fe–N(2) and Fe–CN Reductions

Fe-mediated biological nitrogen fixation is thought to proceed via either a sequence of proton and electron transfer steps, concerted H atom transfer steps, or some combination thereof. Regardless of the specifics and whether the intimate mechanism for N(2)-to-NH(3) conversion involves a distal path...

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Shranjeno v:
Bibliografske podrobnosti
izdano v:J Am Chem Soc
Main Authors: Rittle, Jonathan, Peters, Jonas C.
Format: Artigo
Jezik:Inglês
Izdano: 2017
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC5517100/
https://ncbi.nlm.nih.gov/pubmed/28140600
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b12861
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