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Rhodium-Catalyzed Enantioselective Silylation of Cyclopropyl C-H Bonds
We describe an enantioseleclive silylation of cyclopropanes catalyzed by a rhodium precursor and the bisphosphine (S)-DTBM-SEGPHOS. (Hydrido)silyl ethers, generated in situ by the dehydrogenative silylation of cyclopropylmethanols with diethylsilane, undergo asymmetric, intramolecular silylation of...
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| Publicado no: | Angew Chem Int Ed Engl |
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| Main Authors: | , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4976637/ https://ncbi.nlm.nih.gov/pubmed/27253898 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201603153 |
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