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Reversal of the Regiochemistry in the Rhodium-Catalyzed [4+3] Cycloaddition Between Vinyldiazoacetates and Dienes
A regio-, diastereo- and enantioselective [4+3] cycloaddition between vinylcarbenes and dienes has been achieved using the dirhodium tetracarboxylate catalyst Rh(2)(S-BTPCP)(4). This methodology provides facile access to 1,4-cycloheptadienes that are regioisomers of those formed from the tandem cycl...
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| Publicado en: | Angew Chem Int Ed Engl |
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| Main Authors: | , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado: |
2014
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| Assuntos: | |
| Acceso en liña: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4608551/ https://ncbi.nlm.nih.gov/pubmed/25266984 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201406440 |
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