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Catalytic reduction of N(2) to NH(3) by an Fe-N(2) complex featuring a C-atom anchor

While recent spectroscopic studies have established the presence of an interstitial carbon atom at the center of the iron-molybdenum cofactor (FeMoco) of MoFe-nitrogenase, its role is unknown. We have pursued Fe-N(2) model chemistry to explore a hypothesis whereby this C-atom (previously denoted as...

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Detalhes bibliográficos
Main Authors: Creutz, Sidney E., Peters, Jonas C.
Formato: Artigo
Idioma:Inglês
Publicado em: 2014
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3933546/
https://ncbi.nlm.nih.gov/pubmed/24350667
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja4114962
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