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C—H Bond Cleavage with Reductants: Re-Investigating the Reactivity of Monomeric Mn(III/IV)—Oxo Complexes and the Role of Oxo Ligand Basicity

The thermodynamic properties of structurally similar Mn(III) and Mn(IV) complexes have been re-investigated to understand their reactivity with substrates having C—H bonds. The complexes have the general formula, [MnH(3)buea(O)](n-), where [H(3)buea](3-) is the tripodal ligand, tris[(N’-tert-butylur...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Hauptverfasser: Parsell, Trenton H., Yang, Meng-Yin, Borovik, A. S.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2009
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2787892/
https://ncbi.nlm.nih.gov/pubmed/19196005
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja8100825
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