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Theoretical Analysis of the Unusual Temperature Dependence of the Kinetic Isotope Effect in Quinol Oxidation

This paper presents theoretical calculations on model biomimetic systems for quinol oxidation. In these model systems, an excited-state [Ru(bpy)(2)(pbim)](+) complex (bpy = 2,2’-dipyridyl, pbim = 2-(2-pyridyl)benzimidazolate) oxidizes a ubiquinol or plastoquinol analogue in acetonitrile. The charge...

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Autors principals: Ludlow, Michelle K., Soudackov, Alexander V., Hammes-Schiffer, Sharon
Format: Artigo
Idioma:Inglês
Publicat: 2009
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2710000/
https://ncbi.nlm.nih.gov/pubmed/19351186
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9001184
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