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Theoretical Analysis of the Unusual Temperature Dependence of the Kinetic Isotope Effect in Quinol Oxidation

This paper presents theoretical calculations on model biomimetic systems for quinol oxidation. In these model systems, an excited-state [Ru(bpy)(2)(pbim)](+) complex (bpy = 2,2’-dipyridyl, pbim = 2-(2-pyridyl)benzimidazolate) oxidizes a ubiquinol or plastoquinol analogue in acetonitrile. The charge...

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Detalhes bibliográficos
Main Authors: Ludlow, Michelle K., Soudackov, Alexander V., Hammes-Schiffer, Sharon
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2710000/
https://ncbi.nlm.nih.gov/pubmed/19351186
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9001184
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