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Theoretical Analysis of the Unusual Temperature Dependence of the Kinetic Isotope Effect in Quinol Oxidation

This paper presents theoretical calculations on model biomimetic systems for quinol oxidation. In these model systems, an excited-state [Ru(bpy)(2)(pbim)](+) complex (bpy = 2,2’-dipyridyl, pbim = 2-(2-pyridyl)benzimidazolate) oxidizes a ubiquinol or plastoquinol analogue in acetonitrile. The charge...

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Main Authors: Ludlow, Michelle K., Soudackov, Alexander V., Hammes-Schiffer, Sharon
Format: Artigo
Sprog:Inglês
Udgivet: 2009
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2710000/
https://ncbi.nlm.nih.gov/pubmed/19351186
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja9001184
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