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Diastereo-, Enantio-, and anti-Selective Formation of Secondary Alcohol and Quaternary Carbon Stereocenters by Cu-catalyzed Additions of B-Substituted Allyl Nucleophiles to Carbonyls

A general method for the synthesis of secondary homoallylic alcohols containing α-quaternary carbon stereogenic centers in high diastereo- and enantioselectivity (up to >20:1 dr and >99:1 er) is disclosed. Transformations employ readily accessible aldehydes, allylic diboronates, a chiral coppe...

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Detalhes bibliográficos
Publicado no:Org Lett
Main Authors: Wheatley, Emilie, Zanghi, Joseph M., Meek, Simon J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7797407/
https://ncbi.nlm.nih.gov/pubmed/33206543
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.0c03495
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