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Pd-catalyzed γ-C(sp(3))–H Fluorination of Free Amines

The first example of free amine γ-C(sp(3))–H fluorination is realized using 2-hydroxynicotinaldehyde as the transient directing group. A wide range of cyclohexyl and linear aliphatic amines could be fluorinated selectively at the γ-methyl and methylene positions. Electron withdrawing 3,5-disubstitut...

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Publicat a:J Am Chem Soc
Autors principals: Chen, Yan-Qiao, Singh, Sukriti, Wu, Yongwei, Wang, Zhen, Verma, Pritha, Qiao, Jennifer X., Sunoj, Raghavan B., Yu, Jin-Quan
Format: Artigo
Idioma:Inglês
Publicat: 2020
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC7685760/
https://ncbi.nlm.nih.gov/pubmed/32363869
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b13537
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