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Total Synthesis and Late‐Stage C−H Oxidations of ent‐Trachylobane Natural Products

Herein, we present our studies to construct seven ent‐trachylobane diterpenoids by employing a bioinspired two‐phase synthetic strategy. The first phase provided enantioselective and scalable access to five ent‐trachylobanes, of which methyl ent‐trachyloban‐19‐oate was produced on a 300 mg scale. Du...

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Pubblicato in:Angew Chem Int Ed Engl
Autori principali: Wein, Lukas Anton, Wurst, Klaus, Magauer, Thomas
Natura: Artigo
Lingua:Inglês
Pubblicazione: John Wiley and Sons Inc. 2021
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC7612322/
https://ncbi.nlm.nih.gov/pubmed/34762359
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202113829
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