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Interception of the “Bycroft-Gowland” intermediate in the enzymatic macrocyclization of thiopeptides

Thiopeptides are a broad class of macrocyclic, heavily modified peptide natural products that are unified by the presence of a substituted, nitrogen-containing heterocycle core. Early work indicated that this core might be fashioned from two dehydroalanines by an enzyme-catalyzed aza-[4+2] cycloaddi...

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Détails bibliographiques
Publié dans:J Am Chem Soc
Auteurs principaux: Bogart, Jonathan W., Kramer, Nicholas J., Turlik, Aneta, Bleich, Rachel M., Catlin, Daniel S., Schroeder, Frank C., Nair, Satish K., Williamson, R. Thomas, Houk, K. N., Bowers, Albert A.
Format: Artigo
Langue:Inglês
Publié: 2020
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC7429253/
https://ncbi.nlm.nih.gov/pubmed/32609512
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c05639
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