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Autocatalytic Carbonyl Arylation through In Situ Release of Aryl Nucleophiles from N‐Aryl‐N′‐Silyldiazenes

A method for the catalytic generation of functionalized aryl alkali metals is reported. These highly reactive intermediates are liberated from silyl‐protected aryl‐substituted diazenes by the action of Lewis basic alkali metal silanolates, resulting in desilylation and loss of N(2). Catalytic quanti...

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Bibliografiske detaljer
Udgivet i:Angew Chem Int Ed Engl
Main Authors: Chauvier, Clément, Finck, Lucie, Irran, Elisabeth, Oestreich, Martin
Format: Artigo
Sprog:Inglês
Udgivet: John Wiley and Sons Inc. 2020
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC7383908/
https://ncbi.nlm.nih.gov/pubmed/32030857
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201916004
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