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Enantioselective Allenoate-Claisen Rearrangement Using Chiral Phosphate Catalysts

Herein we report the first highly enantioselective allenoate-Claisen rearrangement using doubly axially chiral phosphate sodium salts as catalysts. This synthetic method provides access to β-amino acid derivatives with vicinal stereocenters in up to 95% ee. We also investigated the mechanism of enan...

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書目詳細資料
發表在:J Am Chem Soc
Main Authors: Miró, Javier, Gensch, Tobias, Ellwart, Mario, Han, Seo-Jung, Lin, Hsin-Hui, Sigman, Matthew S., Toste, F. Dean
格式: Artigo
語言:Inglês
出版: 2020
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC7204274/
https://ncbi.nlm.nih.gov/pubmed/32182422
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c01637
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