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Vinyl Cation Stabilization by Silicon Enables a Formal Metal‐Free α‐Arylation of Alkyl Ketones

The ability of silicon to stabilize vinyl cationic species leads to a redox arylation of alkynes whereby the stringent limitations of reactivity and regioselectivity of alkyl‐substituted alkynes are lifted. This allows the synthesis of a range of α‐silyl‐α′‐arylketones under mild conditions in good...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Pons, Amandine, Michalland, Jean, Zawodny, Wojciech, Chen, Yong, Tona, Veronica, Maulide, Nuno
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6899746/
https://ncbi.nlm.nih.gov/pubmed/31638738
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201909381
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