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Gold-Catalyzed Hydrofluorination of Electron-Deficient Alkynes: Stereoselective Synthesis of β-Fluoro Michael Acceptors

The gold(I)-catalyzed, stereoselective hydrofluorination of electron-deficient alkynes with triethylamine trihydrogen fluoride (Et(3)N·3HF) is described. Fluorinated α,β-unsaturated aldehydes, amides, esters, ketones, and nitriles were isolated in moderate to good yields as single diastereomers. In...

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Detalhes bibliográficos
Publicado no:ACS Catal
Main Authors: O’Connor, Thomas J., Toste, F. Dean
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6874379/
https://ncbi.nlm.nih.gov/pubmed/31763055
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acscatal.8b01341
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