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Oxidant speciation and anionic ligand effects in the gold-catalyzed oxidative coupling of arenes and alkynes

The mechanism of the gold-catalyzed oxidative cross-coupling of arenes and alkynes has been studied in detail combining stoichiometric experiments with putative reaction intermediates and DFT calculations. Our data suggest that ligand exchange between the alkyne, the Au(i)-catalyst and the hypervale...

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Publicado en:Chem Sci
Main Authors: Hofer, Manuel, de Haro, Teresa, Gómez-Bengoa, Enrique, Genoux, Alexandre, Nevado, Cristina
Formato: Artigo
Idioma:Inglês
Publicado: Royal Society of Chemistry 2019
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC6844217/
https://ncbi.nlm.nih.gov/pubmed/31803420
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc02372k
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