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Oxidant speciation and anionic ligand effects in the gold-catalyzed oxidative coupling of arenes and alkynes

The mechanism of the gold-catalyzed oxidative cross-coupling of arenes and alkynes has been studied in detail combining stoichiometric experiments with putative reaction intermediates and DFT calculations. Our data suggest that ligand exchange between the alkyne, the Au(i)-catalyst and the hypervale...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Hofer, Manuel, de Haro, Teresa, Gómez-Bengoa, Enrique, Genoux, Alexandre, Nevado, Cristina
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6844217/
https://ncbi.nlm.nih.gov/pubmed/31803420
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc02372k
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