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Regio- and Enantioselective Synthesis of 1,2-Diamine Derivatives by Copper-Catalyzed Hydroamination

A highly regio- and enantioselective synthesis of 1,2-diamine derivatives from γ-substituted allylic pivalamides using copper-catalyzed hydroamination is reported. The N-pivaloyl group is essential, both in facilitating the hydrocupration step and suppressing an unproductive β-elimination from the a...

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Publicat a:Org Lett
Autors principals: Ichikawa, Saki, Dai, Xi-Jie, Buchwald, Stephen L.
Format: Artigo
Idioma:Inglês
Publicat: 2019
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6825330/
https://ncbi.nlm.nih.gov/pubmed/31099584
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.9b01592
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