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Cobalt Superoxo and Alkylperoxo Complexes Derived from Reaction of Ring-Cleaving Dioxygenase Models with O(2)
The syntheses and O(2) reactivities of active-site models of cobalt-substituted ring-cleaving dioxygenases are presented. The pentacoordinate cobalt(II)-aminophenolate complex, [Co(Tp(Me2))((tBu2)APH)], gives rise to two distinct dioxygen adducts at reduced temperatures. The first is a paramagnetic...
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| 發表在: | J Am Chem Soc |
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| Main Authors: | , , |
| 格式: | Artigo |
| 語言: | Inglês |
| 出版: |
2019
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| 主題: | |
| 在線閱讀: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6748656/ https://ncbi.nlm.nih.gov/pubmed/31251607 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b05320 |
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