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Quantum Suppression of Intramolecular Deuterium Kinetic Isotope Effects in a Pericyclic Hydrogen Transfer Reaction

It is generally accepted that hydrogen tunneling enhances both primary and secondary H/D kinetic isotope effects (KIEs) over what would be expected under the assumptions of classical barrier transition. Previous studies have exclusively shown that the effects of tunneling upon primary H/D KIEs have...

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Publicat a:J Phys Chem A
Autors principals: Li, Xiao, York, Darrin M., Meyer, Matthew P.
Format: Artigo
Idioma:Inglês
Publicat: 2019
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6661151/
https://ncbi.nlm.nih.gov/pubmed/30855141
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpca.9b00172
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