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Quantum Suppression of Intramolecular Deuterium Kinetic Isotope Effects in a Pericyclic Hydrogen Transfer Reaction

It is generally accepted that hydrogen tunneling enhances both primary and secondary H/D kinetic isotope effects (KIEs) over what would be expected under the assumptions of classical barrier transition. Previous studies have exclusively shown that the effects of tunneling upon primary H/D KIEs have...

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Bibliografiska uppgifter
I publikationen:J Phys Chem A
Huvudupphovsmän: Li, Xiao, York, Darrin M., Meyer, Matthew P.
Materialtyp: Artigo
Språk:Inglês
Publicerad: 2019
Ämnen:
Länkar:https://ncbi.nlm.nih.gov/pmc/articles/PMC6661151/
https://ncbi.nlm.nih.gov/pubmed/30855141
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpca.9b00172
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