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An S = 1/2 Iron Complex Featuring N(2), Thiolate, and Hydride Ligands: Reductive Elimination of H(2) and Relevant Thermochemical Fe−H Parameters

Believed to accumulate on the Fe sites of the FeMo-cofactor (FeMoco) of MoFe-nitrogenase under turnover, strongly donating hydrides have been proposed to facilitate N(2) binding to Fe and may also participate in the hydrogen evolution process concomitant to nitrogen fixation. Here, we report the syn...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Gu, Nina X., Oyala, Paul H., Peters, Jonas C.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6592702/
https://ncbi.nlm.nih.gov/pubmed/29684269
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b02603
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