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Chemical Consequences of the Mechanical Bond: A Tandem Active Template‐Rearrangement Reaction
We report the unexpected discovery of a tandem active template CuAAC‐rearrangement process, in which N(2) is extruded on the way to the 1,2,3‐triazole product to give instead acrylamide rotaxanes. Mechanistic investigations suggest this process is dictated by the mechanical bond, which stabilizes th...
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| 出版年: | Angew Chem Int Ed Engl |
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| 主要な著者: | , , , |
| フォーマット: | Artigo |
| 言語: | Inglês |
| 出版事項: |
John Wiley and Sons Inc.
2019
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| 主題: | |
| オンライン･アクセス: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6589916/ https://ncbi.nlm.nih.gov/pubmed/30600892 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201813950 |
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