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Changes in Regioselectivity of H Atom Abstraction during the Hydroxylation and Cyclization Reactions Catalyzed by Hyoscyamine 6β-Hydroxylase

Hyoscyamine 6β-hydroxylase (H6H) is an αKG-dependent nonheme iron oxidase that catalyzes the oxidation of hyoscyamine to scopolamine via two separate reactions: hydroxylation followed by oxidative cyclization. Both of these reactions are expected to involve H atom abstraction from each of two adjace...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Ushimaru, Richiro, Ruszczycky, Mark W., Liu, Hung-wen
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6488026/
https://ncbi.nlm.nih.gov/pubmed/30545219
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b11585
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