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Total Synthesis Establishes the Biosynthetic Pathway to the Naphterpin and Marinone Natural Products

The naphterpins and marinones are naphthoquinone meroterpenoids with an unusual aromatic oxidation pattern that is biosynthesized from 1,3,6,8-tetrahydroxynaphthalene (THN). We propose that cryptic halogenation of THN derivatives by vanadium-dependent chloroperoxidase (VCPO) enzymes is key to this b...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Murray, Lauren A. M., McKinnie, Shaun M. K., Pepper, Henry P., Erni, Reto, Miles, Zachary D., Cruickshank, Michelle C., López-Pérez, Borja, Moore, Bradley S., George, Jonathan H.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
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Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6248334/
https://ncbi.nlm.nih.gov/pubmed/29935040
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201804351
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