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Total Synthesis Establishes the Biosynthetic Pathway to the Naphterpin and Marinone Natural Products

The naphterpins and marinones are naphthoquinone meroterpenoids with an unusual aromatic oxidation pattern that is biosynthesized from 1,3,6,8-tetrahydroxynaphthalene (THN). We propose that cryptic halogenation of THN derivatives by vanadium-dependent chloroperoxidase (VCPO) enzymes is key to this b...

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Publicat a:Angew Chem Int Ed Engl
Autors principals: Murray, Lauren A. M., McKinnie, Shaun M. K., Pepper, Henry P., Erni, Reto, Miles, Zachary D., Cruickshank, Michelle C., López-Pérez, Borja, Moore, Bradley S., George, Jonathan H.
Format: Artigo
Idioma:Inglês
Publicat: 2018
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6248334/
https://ncbi.nlm.nih.gov/pubmed/29935040
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201804351
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