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Terminal Alkyne Coupling Reactions through a Ring: Mechanistic Insights and Regiochemical Switching

The mechanism and selectivity of terminal alkyne coupling reactions promoted by rhodium(I) complexes of NHC‐based CNC pincer ligands have been investigated. Synthetic and kinetic experiments support E‐ and gem‐enyne formation through a common reaction sequence involving hydrometallation and rate‐det...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Storey, Caroline M., Gyton, Matthew R., Andrew, Rhiann E., Chaplin, Adrian B.
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6175324/
https://ncbi.nlm.nih.gov/pubmed/30004163
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201807028
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