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Catalytic Enantioselective Synthesis of Guvacine Derivatives through [4 + 2] Annulations of Imines with α-Methylallenoates

P-Chiral [2.2.1] bicyclic phosphines (HypPhos catalysts) have been applied to reactions between α-alkylallenoates and imines, producing guvacine derivatives. These HypPhos catalysts were assembled from trans-4-hydroxyproline, with the modular nature of the synthesis allowing variations of the exocyc...

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Detalhes bibliográficos
Publicado no:Org Lett
Main Authors: Xu, Qihai, Dupper, Nathan J., Smaligo, Andrew J., Fan, Yi Chiao, Cai, Lingchao, Wang, Zhiming, Langenbacher, Adam D., Chen, Jau-Nian, Kwon, Ohyun
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
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Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6173629/
https://ncbi.nlm.nih.gov/pubmed/30246538
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.8b02489
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