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Fe-Mediated Nitrogen Fixation with a Metallocene Mediator: Exploring pK(a) Effects and Demonstrating Electrocatalysis
Substrate selectivity in reductive multi-electron/proton catalysis with small molecules such as N(2), CO(2), and O(2) is a major challenge for catalyst design, especially where the competing hydrogen evolution reaction (HER) is thermodynamically and kinetically competent. One common strategy to achi...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2018
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6071328/ https://ncbi.nlm.nih.gov/pubmed/29669205 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b02335 |
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