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Catalytic N(2)-to-NH(3) Conversion by Fe at Lower Driving Force: A Proposed Role for Metallocene-Mediated PCET
[Image: see text] We have recently reported on several Fe catalysts for N(2)-to-NH(3) conversion that operate at low temperature (−78 °C) and atmospheric pressure while relying on a very strong reductant (KC(8)) and acid ([H(OEt(2))(2)][BAr(F)(4)]). Here we show that our original catalyst system, P(...
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| Publicado no: | ACS Cent Sci |
|---|---|
| Main Authors: | , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
American Chemical Society
2017
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| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5364448/ https://ncbi.nlm.nih.gov/pubmed/28386599 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acscentsci.7b00014 |
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