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Electrophile-promoted Fe-to-N(2) hydride migration in highly reduced Fe(N(2))(H) complexes

One of the emerging challenges associated with developing robust synthetic nitrogen fixation catalysts is the competitive formation of hydride species that can play a role in catalyst deactivation or lead to undesired hydrogen evolution reactivity (HER). It is hence desirable to devise synthetic sys...

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Publicado en:Chem Sci
Main Authors: Deegan, Meaghan M., Peters, Jonas C.
Formato: Artigo
Idioma:Inglês
Publicado: Royal Society of Chemistry 2018
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC6063139/
https://ncbi.nlm.nih.gov/pubmed/30123481
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c8sc02380h
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