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Spectroscopic Investigations of Catalase Compound II: Characterization of an Iron(IV) Hydroxide Intermediate in a Non-thiolate-Ligated Heme Enzyme

We report on the protonation state of Helicobacter pylori catalase compound II. UV/visible, Mössbauer, and X-ray absorption spectroscopies have been used to examine the intermediate from pH 5 to 14. We have determined that HPC-II exists in an iron(IV) hydroxide state up to pH 11. Above this pH, the...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Yosca, Timothy H., Langston, Matthew C., Krest, Courtney M., Onderko, Elizabeth L., Grove, Tyler L., Livada, Jovan, Green, Michael T.
Formato: Artigo
Idioma:Inglês
Publicado em: 2016
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Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5987761/
https://ncbi.nlm.nih.gov/pubmed/27960340
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b09693
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