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α-Silyl Amides: Effective Bifunctional Lynchpins for Type I Anion Relay Chemistry

Lynchpins comprising α-silyl amides have been validated for type I anion relay chemistry (ARC) to permit ready access to γ-ketoamides. Importantly, the ARC protocol can be run at ambient temperature without the need of additional reagents to trigger the [1,4] Brook rearrangement.

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Bibliografische gegevens
Gepubliceerd in:Org Lett
Hoofdauteurs: Montgomery, Thomas D., Smith, Amos B.
Formaat: Artigo
Taal:Inglês
Gepubliceerd in: 2017
Onderwerpen:
Online toegang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5712993/
https://ncbi.nlm.nih.gov/pubmed/29120188
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.7b03142
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