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Re(2)O(7)-Mediated Dehydrative Cyclization Reactions: Total Synthesis of Herboxidiene and Its 12-Desmethyl Analog

Re(2)O(7) catalysis effects efficient and stereoselective dehydrative cyclization reactions from monoallylic diols, with stereocontrol arising from thermodynamic equilibration. This method was applied to a rapid synthesis of the spliceosome inhibitor herboxidiene. The route was also utilized for the...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Rohrs, Tyler M., Qin, Qi, Floreancig, Paul E.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5687070/
https://ncbi.nlm.nih.gov/pubmed/28686815
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201705924
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