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Two Dynamical Regimes of the Substrate Radical Rearrangement Reaction in B(12)-Dependent Ethanolamine Ammonia-Lyase Resolve Contributions of Native Protein Configurations and Collective Configurational Fluctuations to Catalysis
The kinetics of the substrate radical rearrangement reaction step in B(12)-dependent ethanolamine ammonia-lyase (EAL) from Salmonella typhimurium are measured over a 92 K temperature range. The observed first-order rate constants display a piecewise-continuous Arrhenius dependence, with linear regio...
में बचाया:
| में प्रकाशित: | Biochemistry |
|---|---|
| मुख्य लेखकों: | , , |
| स्वरूप: | Artigo |
| भाषा: | Inglês |
| प्रकाशित: |
2017
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| विषय: | |
| ऑनलाइन पहुंच: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5585081/ https://ncbi.nlm.nih.gov/pubmed/28548844 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.biochem.7b00294 |
| टैग : |
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