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Acyclic quaternary centers from asymmetric conjugate addition of alkylzirconium reagents to linear trisubstituted enones

Synthetic methods for the selective formation of all carbon quaternary centres in non-cyclic systems are rare. Here we report highly enantioselective Cu-catalytic asymmetric conjugate addition of alkylzirconium species to twelve different acyclic trisubstituted enones. A variety of sp(3)-hybridized...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Gao, Zhenbo, Fletcher, Stephen P.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5358539/
https://ncbi.nlm.nih.gov/pubmed/28451211
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc02811j
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