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Critical Aspects of Heme–Peroxo–Cu Complex Structure and Nature of Proton Source Dictate Metal–O(peroxo) Breakage versus Reductive O–O Cleavage Chemistry
The 4H(+)/4e(−) reduction of O(2) to water, a key fuel-cell reaction also carried out in biology by oxidase enzymes, includes the critical O–O bond reductive cleavage step. Mechanistic investigations on active-site model compounds, which are synthesized by rational design to incorporate systematic v...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5274545/ https://ncbi.nlm.nih.gov/pubmed/28029788 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b11322 |
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