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Does the pressure dependence of kinetic isotope effects report usefully on dynamics in enzyme H‐transfer reactions?

The temperature dependence of kinetic isotope effects (KIEs) has emerged as the main experimental probe of enzymatic H‐transfer by quantum tunnelling. Implicit in the interpretation is a presumed role for dynamic coupling of H‐transfer chemistry to the protein environment, the so‐called ‘promoting m...

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Detalhes bibliográficos
Publicado no:FEBS J
Main Authors: Hoeven, Robin, Heyes, Derren J., Hay, Sam, Scrutton, Nigel S.
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4949571/
https://ncbi.nlm.nih.gov/pubmed/25581554
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1111/febs.13193
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