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Total Synthesis of Gelsenicine via a Catalyzed Cycloisomerization Strategy
The first total synthesis of (±)-gelsenicine is reported. The synthetic route is highly efficient (13 steps), featuring (1) a pivotal metal-catalyzed isomerization/rearrangement process that forges the central core of the molecule and (2) two facile C–N bond-forming steps that establish the flanking...
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| Gepubliceerd in: | J Am Chem Soc |
|---|---|
| Hoofdauteurs: | , , , |
| Formaat: | Artigo |
| Taal: | Inglês |
| Gepubliceerd in: |
2015
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| Onderwerpen: | |
| Online toegang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4732274/ https://ncbi.nlm.nih.gov/pubmed/26716762 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b12263 |
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