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Total Synthesis of Gelsenicine via a Catalyzed Cycloisomerization Strategy

The first total synthesis of (±)-gelsenicine is reported. The synthetic route is highly efficient (13 steps), featuring (1) a pivotal metal-catalyzed isomerization/rearrangement process that forges the central core of the molecule and (2) two facile C–N bond-forming steps that establish the flanking...

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Bibliografski detalji
Izdano u:J Am Chem Soc
Glavni autori: Newcomb, Eric T., Knutson, Phil C., Pedersen, Blaine A., Ferreira, Eric M.
Format: Artigo
Jezik:Inglês
Izdano: 2015
Teme:
Online pristup:https://ncbi.nlm.nih.gov/pmc/articles/PMC4732274/
https://ncbi.nlm.nih.gov/pubmed/26716762
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b12263
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