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Evidence for an oxygen evolving iron–oxo–cerium intermediate in iron-catalysed water oxidation
The non-haem iron complex α-[Fe(II)(CF(3)SO(3))(2)(mcp)] (mcp = (N,N′-dimethyl-N,N′-bis(2-pyridylmethyl)-1,2-cis-diaminocyclohexane) reacts with Ce(IV) to oxidize water to O(2), representing an iron-based functional model for the oxygen evolving complex of photosystem II. Here we trap an intermediat...
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| Publicado no: | Nat Commun |
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| Main Authors: | , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2015
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4722336/ https://ncbi.nlm.nih.gov/pubmed/25609387 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/ncomms6865 |
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