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Rhodium-Catalyzed Enantioselective Silylation of Arene C–H Bonds: Desymmetrization of Diarylmethanols

We report a Rh-catalyzed, enantioselective silylation of arene C–H bonds directed by a (hydrido)silyl group. (Hydrido)silyl ethers that are formed in situ by hydrosilylation of benzophenone or its derivatives undergo asymmetric C–H silylation in high yield with excellent enantioselectivity in the pr...

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Détails bibliographiques
Publié dans:J Am Chem Soc
Auteurs principaux: Lee, Taegyo, Wilson, Tyler W., Berg, Robert, Ryberg, Per, Hartwig, John F.
Format: Artigo
Langue:Inglês
Publié: 2015
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC4699421/
https://ncbi.nlm.nih.gov/pubmed/25948056
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b03091
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