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Enantioselective Ruthenium Catalyzed Carbonyl Allylation via Alkyne-Alcohol C-C Bond Forming Transfer Hydrogenation: Allene Hydrometallation vs. Oxidative Coupling

Chiral ruthenium(II) complexes modified by Josiphos ligands catalyze the reaction of alkynes with primary alcohols to form homoallylic alcohols with excellent control of regio-, diastereo- and enantioselectivity. These processes represent the first examples of enantioselective carbonyl allylation us...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Liang, Tao, Nguyen, Khoa D., Zhang, Wandi, Krische, Michael J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4385519/
https://ncbi.nlm.nih.gov/pubmed/25734220
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b00747
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