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Crystal structures of alkylperoxo and anhydride intermediates in an intradiol ring-cleaving dioxygenase
Intradiol aromatic ring-cleaving dioxygenases use an active site, nonheme Fe(3+) to activate O(2) and catecholic substrates for reaction. The inability of Fe(3+) to directly bind O(2) presents a mechanistic conundrum. The reaction mechanism of protocatechuate 3,4-dioxygenase is investigated here usi...
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| Udgivet i: | Proc Natl Acad Sci U S A |
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| Main Authors: | , , |
| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
National Academy of Sciences
2015
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4299229/ https://ncbi.nlm.nih.gov/pubmed/25548185 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1419118112 |
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