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Structural dynamics inside a functionalized metal–organic framework probed by ultrafast 2D IR spectroscopy
The structural elasticity of metal–organic frameworks (MOFs) is a key property for their functionality. Here, we show that 2D IR spectroscopy with pulse-shaping techniques can probe the ultrafast structural fluctuations of MOFs. 2D IR data, obtained from a vibrational probe attached to the linkers o...
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| Publicado en: | Proc Natl Acad Sci U S A |
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| Autores principales: | , , , , , , |
| Formato: | Artigo |
| Lenguaje: | Inglês |
| Publicado: |
National Academy of Sciences
2014
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| Materias: | |
| Acceso en línea: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4284562/ https://ncbi.nlm.nih.gov/pubmed/25512539 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1422194112 |
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