Observation of a Cu(II)(2)(μ-1,2-peroxo)/Cu(III)(2)(μ-oxo)(2) Equilibrium and its Implications for Copper-Dioxygen Reactivity()

Synthesis of small molecule Cu(2)O(2) adducts has provided insight into the related biological systems and their reactivity patterns including the interconversion of the Cu(II)(2)(μ-η(2):η(2)-peroxo) and Cu(III)(2)(μ-oxo)(2) isomers. In this study, absorption spectroscopy, kinetics, and resonance Ra...

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Main Authors: Kieber-Emmons, Matthew T., Ginsbach, Jake W., Wick, Patrick K., Lucas, Heather R., Helton, Matthew E., Lucchese, Baldo, Suzuki, Masatatsu, Zuberbühler, Andreas, Karlin, Kenneth D., Solomon, Edward I.
Formato: Artigo
Idioma:Inglês
Publicado em: 2014
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Article
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4041702/
https://ncbi.nlm.nih.gov/pubmed/24700427
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201402166
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