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Nature-Inspired Stereospecific Total Synthesis of P-(+)-Dispegatrine as well as the Total Synthesis of Four Other Monomeric Sarpagine Indole Alkaloids

Non-phenolic oxidative coupling: The first total synthesis of the C-2 symmetric indole alkaloid P-(+)-dispegatrine (1) is reported. A late-stage thallium(III)acetate mediated intermolecular oxidative coupling was employed to construct the C(9)-C(9′) bond with complete regio- and stereocontrol. The e...

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Detalles Bibliográficos
Main Authors: Edwankar, Chitra R., Edwankar, Rahul V., Deschamps, Jeffrey R., Cook, James M.
Formato: Artigo
Idioma:Inglês
Publicado: 2012
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC3970238/
https://ncbi.nlm.nih.gov/pubmed/23073985
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201206015
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