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EPR and Mössbauer Spectroscopy, and DFT Analysis of a High-Spin Fe(IV)-oxo Complex

The kinetically competent oxidant in non-heme iron enzymes is a high-spin Fe(IV)-oxo species, which are not as well characterized as the intermediate-spin species of heme systems. The present work gives a detailed characterization of the structurally similar [Fe(IV)H(3)buea(O)](-), [Fe(III)H(3)buea(...

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Bibliografiske detaljer
Main Authors: Gupta, Rupal, Lacy, David C., Bominaar, Emile L., Borovik, Andrew. S., Hendrich, Michael P.
Format: Artigo
Sprog:Inglês
Udgivet: 2012
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3869391/
https://ncbi.nlm.nih.gov/pubmed/22574962
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja303224p
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